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Top-down approaches

Thompson, Rona Louise; Chevallier, Frédéric; Maksyutov, Shamil; Patra, Prabir K.; Bowman, Kevin

2022

Top-down assessment of air pollution and GHGs for Dhaka, Bangladesh. Analysis of GAINS derived model data. NILU TR

Randall, S.

The city of Dhaka was chosen for this assessment due to the current ongoing project Bangladesh Air Pollution Management (BAPMAN), which concentrates mostly on the capital city Dhaka. The Greenhouse Gas and Air Pollution Interactions and Synergies model (GAINS) was used to performed this top-down assessment due to the models integrated assessment approach of capturing interactions between air pollution control and economic development, as well as its focus on presenting cost effective pollution control strategies. Results from the GAINS model assessment for Dhaka shows that for 2010 the total PM2.5 emissions were 35000 tons/year, and the total PM10 emissions were 45000 tons/year. The top sectors making up the PM emissions included Industry and Residential sectors, where the specific sub-sectors were brick/cement production and residential cooking respectively; the top activities making up the emissions were 'no fuel use' and 'fuelwood direct'. GAINS estimates that the top 3 technical control measures available for PM can eliminate approximately 1/3 of the PM emissions at a cost of .65 MEuro/year. GAINS results also shows that for Dhaka in 2010 the total SO2 emissions were 34000 tons/year, dominated by the Industrial sector, made up of the sub-sectors of new power plants and industrial combustion; top activities contributing to these emissions are hard coal and natural gas. NOX emissions for Dhaka in 2010 were 30000 tons/year, dominated by the Industrial and Transport sectors, made up of the industrial combustion/power plant and light/heavy duty sub-sectors respectively; top activities contributing to these emissions include natural gas, gasoline, and medium distillates. GHG emissions for Dhaka in 2010 exceeded 23 million tons/year, dominated by the Industrial and Agricultural sectors, comprising of the industrial combustion and new power plant sub-sectors; top activities contributing to these emissions include natural gas and hard coal.

2011

Top-down assessment of the Asia carbon budget since the mid 1990s.

Canadell, P.; Thompson, R. L.; Patra, P.; Chevallier, F.; Maksyutov, S.; Law, R.; Ziehn, T.; van der Laan-Luijkx, I.; Peters, W.; Ganshin, A.; Zhuravlev, R.; Maki, T.; Nakamura, T.; Shirai, T.; Poulter, B.; Ciais, P.

2015

Top-down assessment of the Asian carbon budget since the mid 1990s.

Thompson, R.L.; Patra, P.K.; Chevallier, F.; Maksyutov, S.; Law, R.M.; Ziehn, T.; van der Laan-Luijkx, I.T.; Peters, W.; Ganshin, A.; Zhuravlev, R.; Maki, T.; Nakamura, T.; Shirai, T.; Ishizawa, M.; Saeki, T.; Machida, T.; Poulter, B.; Canadell, J.G.; Ciais, P.

2016

Top-down constraints on atmospheric mercury emissions and implications for global biogeochemical cycling.

Song, S.; Selin, N.E.; Soerensen, A.L.; Angot, H.; Artz, R.; Brooks, S.; Brunke, E.-G.; Conley, G.; Dommergue, A.; Ebinghaus, R.; Holsen, T.M.; Jaffe, D.A.; Kang, S.; Kelley, P.; Luke, W. T.; Magand, O.; Marumoto, K.; Pfaffhuber, K.A.; Ren, X.; Sheu, G.-R.; Slemr, F.; Warneke, T.; Weigelt, A.; Weiss-Penzias, P.; Wip, D.C.; Zhang, Q.

2015

Top-down estimate of methane fluxes in Siberia in 2020

Marthinsen, Erik; Thompson, Rona Louise; Pisso, Ignacio; Westermann, Sebastian; Müller, Jurek; Sasakawa, Motoki; Zaehle, Sönke

2023

Top-down estimates of benzene and toluene emissions in the Pearl River Delta and Hong Kong, China.

Fang, X. K.; Shao, M.; Stohl, A.; Zhang, Q.; Zheng, J. Y.; Guo, H.; Wang, C.; Wang, M.; Ou, J. M.; Thompson, R. L.; Prinn, R. G.

2016

Top-down estimates of European CH4 and N2O emissions based on four different inverse models.

Bergamaschi, P.; Corazza, M.; Karstens, U.; Athanassiadou, M.; Thompson, R.L.; Pison, I.; Manning, A.J.; Bousquet, P.; Segers, A.; Vermeulen, A.T.; Janssens-Maenhout, G.; Schmidt, M.; Ramonet, M.; Meinhardt, F.; Aalto, T.; Haszpra, L.; Moncrieff, J.; Popa, M.E.; Lowry, D.; Steinbacher, M.; Jordan, A.; O'Doherty, S.; Piacentino, S.; Dlugokencky, E.

2014

Top-down estimates of European CH4 and N2O emissions based on four different inverse models.

Bergamaschi, P.; Corazza, M.; Karstens, U.; Athanassiadou, M.; Thompson, R. L.; Pison, I.; Manning, A. J.; Bousquet, P.; Segers, A.; Vermeulen, A. T.; Janssens-Maenhout, G.; Schmidt, M.; Ramonet, M.; Meinhardt, F.; Aalto, T.; Haszpra, L.; Moncrieff, J.; Popa, M. E.; Lowry, D.; Steinbacher, M.; Jordan, A.; O'Doherty, S.; Piacentino, S.; Dlugokencky, E.

2015

Top-down estimates of N2O emissions over the past two decades

Thompson, Rona Louise; Lassaletta, Luis; Patra, Prabir; Wilson, C.; Wells, Kelley C.; Gressent, Alicia; Koffi, Ernest; Chipperfield, M. P; Winiwarter, Wilfried; Davidson, E. A.; Tian, H.; Canadell, P.

2019

Top-down estimates of N2O emissions over the past two decades

Thompson, Rona Louise; Wells, Kelley C.; Wilson, Chris J.; Gressent, Alicia; Koffi, Ernest; Bergamaschi, Peter; Millet, Dylan B.; Patra, Prabir Kumar; Prather, Michael J.; Tian, Hanqin; Suntharalingam, Parvadha; Canadell, Josep Gili

2018

Top-down validation of global and East Asian emissions of tetrafluoromethane and hexaflurorethane. NILU F

Kim, J.; Muhle, J.; Fraser, P.J.; Li, S.; Arnold, T.; Harth, C.M.; Salameh, P.; Steele, P.; Krummel, P.B.; Leist, M.; Stohl, A.; Park, M.; Weiss, R.F.; Kim, K.

2010

TOR: An Overview of Tropospheric Ozone Research Transport and Chemical Transformation of Pollutants in the Troposphere, 3373, vol. 1

Hov, Ø.; Kley, D.; Volz-Thomas, A.; Beck, J.; Grennfelt, P.; Penkett, S.A.

2000

Total deposition of major inorganic ions at non-urban sites in China, 2000-2004 (part II).

Jin, L.; Shao, M.; Aas, W.; Duan, L.; Vogt, R.D.; Zhao, D.; Xiang, R.; Zhang, J.; Xiao, J.

2005

Total deposition of major inorganic ions at non-urban sites in China, 2001-2003 (part II). NILU PP

Jin, L.; Shao, M.; Aas, W.; Duan, L.; Vogt, R.D.; Zhao, D.; Xiang, R.; Zhang, J.; Xiao, J.

2005

Total deposition of major inorganic ions at non-urban sites in China, 2001-2003.

Jin, L.; Shaoi, M.; Aas, W.; Duan, L.; Vogt, R.D.; Zhao, D.; Xiang, J. Zhang, J.; Xiao, J.

2007

Total oxidizable precursors assay for PFAS in human serum

Cioni, Lara; Nikiforov, Vladimir; Miranda Fernandes Coelho, Ana Carolina; Sandanger, Torkjel M; Herzke, Dorte

Per- and polyfluoroalkyl substances (PFAS) are a class of chemicals including over 4700 substances. As a limited number of PFAS is routinely analyzed in human serum, complementary analytical methods are required to characterize the overlooked fraction. A promising tool is the total oxidizable precursors (TOP) assay to look for precursors by oxidation to perfluoroalkyl acids (PFAA). The TOP assay was originally developed for large volumes of water and had to be adapted for 250 μL of human serum. Optimization of the method was performed on serum samples spiked with model precursors. Oxidative conditions similar to previous TOP assay methods were not sufficient for complete oxidation of model precursors. Prolonged heating time (24 h) and higher oxidant amount (95 mg of Na2S2O8 per 225 μL of serum) were needed for complete conversion of the model precursors and accomplishing PFAA yields of 35–100 %. As some precursors are not fully converted to PFAA, the TOP assay can only provide semi-quantitative estimates of oxidizable precursors in human serum. However, the TOP assay can be used to give indications about the identity of unknown precursors by evaluating the oxidation products, including perfluoroalkyl sulfonic acids (PFSA) and perfluoroalkyl ether carboxylic acids (PFECA). The optimized TOP assay for human serum opens the possibility for high-throughput screening of human serum for undetected PFAA precursors.

Elsevier

2022

Total ozone and UV measurements at the Norwegian Troll Station, Antarctica.

Hansen, G.; Svendby, T.; Dahlback, A.; Edvardsen, K.

2016

Total ozone loss during the 2005/2006 Arctic winter and comparison to previous years. Poster presentation. NILU PP

Goutail, F.; Lefèvre, F.; Pommereau, J.P.; van Roozendael, M.; Chipperfield, M.; Feng, W.; Kyro, E.; Andersen, S.B.; Stebel, K.; Dorokhov, V.

2006

Total ozone loss during the 2006/07 Arctic winter and comparison to previous year.

Goutail, F.; Lefèvre, F.; Pommereau, J.P.; Chipperfield, M.; Feng, W.; van Roozendael, M.; Andersen, S.B.; Stebel, K.; Dorokhov, V.; Kyro, E.; Fraser, A.; Strong, K.

2007

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